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          學科建設

          學科建設

          我校化學化工學院在光電功能材料研究領域取得系列重要成果

          時間:2018-12-04瀏覽:10來源:科研處作者:



          化學化工學院“晶體工程”研究團隊成員梅大江老師長期從事無機光電功能材料研究,其中主要包括非線性光學晶體材料以及可見光催化材料,近期取得系列成果,并在國際高水平期刊上發表多篇研究論文。



          在非線性光學晶體材料方面:針對硫化物非線性光學晶體熔點較高,生長比較困難的問題首次提出“低熔點、高性能晶體材料”理論,最終獲得低熔點高性能非線性光學晶體材料LiGaGe2S6。該研究已經申請并授權中國發明專利一項(一種LiGaGe2S6化合物和LiGaGe2S6非線性光學晶體及制備方法與應用ZL201610077818.2);為了提高中紅外非線性光學晶體材料激光損傷閾值,團隊從最大帶隙硼酸鹽氧化物SrB4O7出發,通過第一性原理計算進行預測,設計合成出同時具有良好非線性光學系數和高激光損傷閾值的新型非線性光學晶體材料BaAl4S7。在可見光催化材料方面,針對氧化物可見光催化材料帶隙大,不利于吸收利用可見光的問題,團隊從具有結構多樣性,物理化學性能豐富的金屬硫屬化合物入手,合成了具有更小帶隙的低維新型可見光催化劑Ba6Zn6HfS14,并且在微米級粒徑可見光催化劑中表現出良好的催化性能。


          以上研究成果分別發表于Nature Index 期刊Inorganic Chemistry,題為“LiGaGe2S6: A Chalcogenide with Good Infrared Nonlinear Optical Performance and Low Melting Point”DOI: 10.1021/acs.inorgchem.7b01989,第一作者:梅大江);英國皇家化學學會著名期刊Journal of Materials Chemistry C,題為“Design and synthesis of a nonlinear optical material BaAl4S7 with a wide band gap inspired from SrB4O7” (DOI: 10.1039/c7tc05693a,第一作者:梅大江);美國化學學會著名期刊Crystal Growth & Designs,題為“Rational band design in metal chalcogenide Ba6Zn6HfS14: splitting orbitals, narrowing forbidden gap and boosting photocatalyst property”DOI: 10.1021/acs.cgd.8b01256,第一作者:操汪柱,通訊作者:梅大江)。以上研究獲得國家自然科學基金,稀土資源利用國家重點實驗室開放課題基金,中科院“功能晶體與激光技術”重點實驗室開放課題基金,上海工程技術大學展翅人才計劃,上海高校青年教師培養資助計劃,綠色催化四川省高校重點實驗室開放課題基金,上海工程技術大學科研啟動基金的支持。

            



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